Context. The SDSS-II Supernova Survey, conducted between 2005 and 2007, wasdesigned to detect a large number of Type Ia supernovae (SNe Ia) around z~0.2,the redshift "gap" between low-z and high-z SN searches. The survey hasprovided multi-band photometric lightcurves for variable targets, and SNcandidates were scheduled for spectroscopic observations, primarily to provideSN classification and accurate redshifts. We present SN spectra obtained in2006 and 2007 using the NTT and the NOT. Aims. We provide an atlas of SNspectra in the range z =0.03-0.32 that complements the well-sampled lightcurvesfrom SDSS-II in the forthcoming three-year SDSS SN cosmology analysis. Thesample can, for example, be used for spectral studies of SNe Ia, which arecritical for understanding potential systematic effects when SNe are used todetermine cosmological distances. Methods. The spectra were reduced in auniform manner, and special care was taken in estimating the uncertainties forthe different processing steps. Host-galaxy light was subtracted when possibleand the SN type fitted using the SuperNova IDentification code (SNID). We alsopresent comparisons between spectral and photometric dating using SALTlightcurve fits to the photometry from SDSS-II, as well as the globaldistribution of our sample in terms of the lightcurve parameters: stretch andcolour. Results. We report new spectroscopic data from 141 SNe Ia, mainlybetween -9 and +15 days from lightcurve maximum, including a few cases ofmulti-epoch observations. This homogeneous, host-galaxy subtracted, SN Iaspectroscopic sample is among the largest such data sets and unique in itsredshift interval. The sample includes two potential SN 1991T-like SNe (SN2006on and SN 2007ni) and one potential SN 2002cx-like SN (SN 2007ie). Inaddition, the new compilation includes spectra from 23 confirmed Type II and 8Type Ib/c SNe.